Learn · Organic Chemistry

Addition Reactions of Alkynes

Hydrohalogenation, hydration, and reduction of the triple bond.

Quick answer A triple bond is two π bonds, so reagents can add twice, and oxygen-bearing products tautomerize to carbonyls. Four controls: Markovnikov hydration (H2O, H2SO4, HgSO4) → ketone; hydroboration → aldehyde; H2/Lindlar → cis alkene; Na/NH3trans alkene.
Mechanism · Addition of HBr to Alkynes2 steps
Step 1 — first HBr (Markovnikov).
CH3HHBrCH2CH3Br2-bromopropene
The π bond adds HBr, Markovnikov, to give a vinyl bromide.
Step 2 — second HBr, same carbon.
CH2CH3BrHBrCH3CH3BrBr2,2-dibromopropane
A second HBr adds to the same carbon → geminal dibromide.

Whether hydration gives an aldehyde or a ketone depends on the substrate: a terminal alkyne bears an sp C–H, an internal alkyne buries the triple bond mid-chain.

Acetylene (ethyne)
Propyne (terminal)
2-Butyne (internal)

1. A triple bond is two π bonds, so electrophiles can add twice.

The first addition leaves a still-nucleophilic double bond; equivalents of reagent decide whether you stop there or add again.

2. Hydrohalogenation adds HX with Markovnikov regiochemistry: one equivalent gives a vinyl halide, two give a geminal dihalide.

One equivalent of HX adds Markovnikov (halogen to the more substituted carbon) and stops at a vinyl halide.

Markovnikov addition of one HBr → a vinyl bromide.

A second equivalent adds again Markovnikov, so both halogens land on the same carbon — a geminal dihalide.

Two equivalents drive a second Markovnikov addition to the gem-dibromide.

3. Acid-catalyzed hydration gives a Markovnikov enol that tautomerizes to a ketone.

With H2O, H2SO4, HgSO4, water adds Markovnikov (OH on the more substituted carbon) to give an enol.

Markovnikov hydration of propyne → acetone (via an enol).

The enol immediately tautomerizes to the stable carbonyl, and since OH sat on the more substituted carbon it is a ketone (a methyl ketone from a terminal alkyne).

Enol (unstable)
Ketone (favored tautomer)

4. Hydroboration–oxidation delivers water anti-Markovnikov, turning a terminal alkyne into an aldehyde.

A bulky dialkylborane (R2BH) then H2O2, NaOH puts boron — and OH — on the terminal carbon, giving an anti-Markovnikov enol.

Anti-Markovnikov hydration of propyne → propanal, an aldehyde.

This enol tautomerizes with the oxygen on the terminal carbon, so it becomes an aldehyde — the standard route from a terminal alkyne.

5. Reduction reagents let you choose the cis alkene, the trans alkene, or the alkane.

The reagent sets both how far reduction goes and the geometry:

  • H2, Lindlar catalyst — syn addition stops at the cis (Z) alkene.
  • Na (or Li) in liquid NH3 — dissolving-metal reduction gives the trans (E) alkene.
  • H2, Pd/C — reduces all the way to the alkane.
cis (H2, Lindlar)
trans (Na, NH3)
alkane (H2, Pd/C)

6. Summary

1 eq HX → vinyl halide · 2 eq HX → gem-dihalide · H2O/H2SO4/HgSO4 → ketone · R2BH then H2O2/NaOH → aldehyde · H2/Lindlar → cis · Na/NH3 → trans · H2/Pd-C → alkane.

Worked example

Problem. What is the product of propyne + 2 equivalents of HBr?
  1. HBr adds with Markovnikov orientation: H to the terminal carbon, Br to the internal (more-substituted) carbon → 2-bromopropene.
  2. The second HBr again adds Markovnikov, placing the second Br on the same carbon (now stabilised by the first Br).

Answer. 2,2-dibromopropane (a geminal dihalide).

Quiz yourself

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2,2-Dibromopropane, a geminal dihalide. Both additions are Markovnikov, so both bromines go to the same (more substituted, internal) carbon. One equivalent would stop at the vinyl bromide 2-bromopropene.

Both routes make an enol that tautomerizes to a carbonyl; the difference is where the OH lands. Hg-catalyzed hydration is Markovnikov (OH on the more substituted carbon → ketone). Hydroboration puts boron, and then OH, on the terminal carbon (anti-Markovnikov) → aldehyde.

Use Na (or Li) in liquid NH3 — dissolving-metal reduction gives the trans (E) alkene. For the cis (Z) isomer use H2 with Lindlar catalyst (syn addition). Ordinary H2/Pd-C would overshoot to butane.

A triple bond contains two π bonds. The first addition consumes one π bond and leaves a double bond behind, which still has a π bond available to react with a second equivalent. An alkene starts with only one π bond, so it is saturated after a single addition.

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