Learn · Organic Chemistry

Free-Radical Halogenation of Alkanes

Initiation, propagation, termination — and why Br₂ is more selective than Cl₂.

Quick answer Radical halogenation swaps one C–H for a C–X using X2 + light/heat, running by a radical chain whose hydrogen-abstraction step picks the C–H that gives the most stable radical (3° > 2° > 1° > methyl). Br2 is slow and selective; Cl2 is fast and gives mixtures.
Mechanism · Radical Halogenation3 steps
Initiation — homolyse the halogen.
ClClhv / ΔClCltwo chlorine radicals
Light or heat splits Cl–Cl homolytically (one electron to each atom — shown with single-barbed fishhook arrows), giving two chlorine radicals.
Propagation 1 — abstract a hydrogen.
ClHCH3fishhooks = 1 electron eachClHCH3new carbon radical
A chlorine radical pulls an H off the alkane, forming H–Cl and a new carbon radical. Selectivity follows radical stability: 3° > 2° > 1°.
Propagation 2 — grab a halogen.
CH3ClClCH3ClClproduct + chain carrier
The carbon radical takes a chlorine from Cl2, giving the alkyl halide and regenerating a chlorine radical — which carries the chain forward. (Two radicals combining would be termination.)

Radical halogenation installs the first functional handle on an otherwise inert alkane, and it works through neutral radicals in a self-sustaining chain rather than polar arrows.

The whole reaction in one line: light, a halogen, and one C–H becomes one C–X. Structures drawn live.

1. It Swaps One C–H for One C–X — the Only Reaction Alkanes Reliably Do

Under heat or UV light (hν) an alkane reacts with Cl2 or Br2 to give R–H + X2 → R–X + HX; F2 is too violent and I2 unfavorable.

Ethane plus Cl2 under light gives chloroethane and HCl.

2. It Runs as a Chain: Initiation, Propagation, Termination

Initiation homolytically splits X2 into two X•; propagation is two steps that regenerate a radical (X• grabs H → R• + HX; R• grabs X → R–X + X•); termination pairs any two radicals.

Initiation: hν splits Br2 homolytically into two bromine radicals, Br•.
Propagation 1: Br• abstracts an H from the alkane, giving a carbon radical (an ethyl radical here) and H–Br.
Propagation 2: the carbon radical grabs Br from Br2, forming R–Br and regenerating Br• to continue the chain.

3. The Hydrogen-Abstraction Step Decides Everything

Only the first propagation step — X• abstracting a hydrogen — chooses which C–H reacts, so the product is set by which carbon radical is easiest (most stable) to make.

The carbon radical produced by H-abstraction — its stability sets the selectivity.

4. Radical Stability Follows 3° > 2° > 1° > Methyl

Neighboring alkyl groups donate electron density (hyperconjugation and induction) into the radical center, so more attached carbons means a more stable radical — a 3° C–H is abstracted far more readily than a 1° one.

Methyl (least stable)
Primary (1°)
Secondary (2°)
Tertiary (most stable)

5. Bromination Is Selective; Chlorination Is Not

By the Hammond postulate, endothermic Br• abstraction has a late, radical-like transition state that fully feels stability (one clean product at the most substituted carbon), while exothermic Cl• abstraction has an early one that barely discriminates (mixtures).

Selective bromination of isobutane hits the single 3° C–H → tert-butyl bromide, essentially one product.

Chlorinating propane, by contrast, gives a mixture:

1-chloropropane (from a 1° H)
2-chloropropane (from the 2° H)

6. Allylic and Benzylic C–H Bonds React Fastest of All

A radical next to a C=C (allylic) or aromatic ring (benzylic) is resonance-delocalized, making it even more stable than 3°, so these C–H bonds react fastest — often brominated with NBS.

Allyl radical (resonance-stabilized)
Benzyl radical (resonance-stabilized)

7. Summary

X2 + light swaps one C–H for C–X via a radical chain · H-abstraction is selectivity-determining · stability 3° > 2° > 1° > methyl (allylic/benzylic highest) · Br2 selective, Cl2 gives mixtures.

Methyl
3° — reacts most readily

Quiz yourself

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The first one — X• abstracting a hydrogen from the alkane. It is the step that decides which C–H reacts and forms the carbon radical, so its transition-state energy sets both the rate and the product distribution. The second step (R• grabbing a halogen from X2) is fast and indiscriminate.

3° > 2° > 1° > methyl. More attached alkyl groups donate electron density (hyperconjugation and induction) to the electron-deficient radical center, lowering its energy — the same trend as carbocations. Resonance-stabilized allylic and benzylic radicals are even more stable than 3°.

Br2. Its endothermic H-abstraction has a late, product-like transition state (Hammond postulate) that fully "feels" radical stability, so it strongly favors the most stable radical and gives one dominant product. Cl2 has an early transition state, barely discriminates, and gives mixtures of constitutional isomers.

Because the resulting allylic radical is resonance-stabilized — its unpaired electron delocalizes across the adjacent π bond, spreading over two carbons. That extra delocalization makes it more stable (and its C–H weaker) than a tertiary radical, which is stabilized only by nearby alkyl groups. Benzylic C–H bonds react for the same reason.

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